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London appeared on numerous television series in the 1960s, including guest appearances on Rawhide (1960), Laramie (1960), I Spy (1965), Alfred Hitchcock Presents (1965) and The Big Valley (1968). She and second husband Bobby Troup frequently appeared as panelists on the game shows Tattletales , Hollywood Squares , and Masquerade Party in the 1970s. On May 28, 1964, she and Troup recorded a one-hour program for Japanese television in Japan. London sang 13 of her classic songs, including “Bye Bye Blackbird”, “Lonesome Road”, and “Cry Me a River”. She released studio albums until the end of the decade, and her final studio album was Yummy, Yummy, Yummy (1969), a collection of contemporary songs. After this, London stopped singing professionally. She had lost significant vocal control due to years of smoking and drinking.